Graduate theses
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Title |
Synthesis of AaeUPO polymer bioconjugates |
Author
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Δραμουντάνη, Ειρήνη
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Thesis advisor
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Βελώνια, Καλλιόπη
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Abstract |
Catalysis is among the numerous applications
enzyme polymer conjugates are
expected to find in the field of materials science due to their ability to enhance
and/or differentiate the activity of the parent enzymes. In this report, the
synthesis of protein polymer conjugates of AaeUPO, a peroxygenase isolat ed
from the basidiomycete Agrocybe aegerita , is presented. Peroxygenases have
drawn significant interest as 450 monooxygenase substitutes. As heme thiolate
enzymes, their range of reactions resembles that of P450 monooxygenases
however, peroxygenases utili ze hydrogen peroxide or organic peroxides as
oxidants, which enables their application also in non aqueous media.
Therefore, UPOs are attractive biocatalysts for selective oxyfunctionalization of
otherwise non reactive carbons. A variety of monomers were u tilized to
synthesize hydrophobic, hydrophilic, responsive protein polymer bioconjugates
via oxygen tolerant , controlled radical polymerization The
synthesis and characterization of a variety of such bioconjugates will be
presented together wit h initial studies on their response and catalytic properties.
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Language |
Greek |
Subject |
Peroxygenase |
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UPO |
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bioconjugates |
Issue date |
2023-07-19 |
Collection
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School/Department--School of Sciences and Engineering--Department of Materials Science and Technology--Graduate theses
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Type of Work--Graduate theses
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Permanent Link |
https://elocus.lib.uoc.gr//dlib/0/2/d/metadata-dlib-1696488987-302402-21235.tkl
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Views |
413 |
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