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Identifier 000457376
Title Design and development of novel metal-organic frameworks with tunable guest responsive properties
Alternative Title Σχεδιασμός και ανάπτυξη καινοτόμων Μεταλλο-Οργανικών Πλεγμάτων με ελεγχόμενες ιδιότητες απόκρισης σε εξωτερικά ερεθίσματα
Author Παπαδόπουλος, Κωνσταντίνος Γεωρ.
Thesis advisor Τρικαλίτης, Παντελής
Reviewer Μήλιος, Κωνσταντίνος
Φρουδάκης, Γεώργιος
Abstract MOFs are unique solid-state materials and their advantage over traditional porous materials lies in the fact that they are composed of organic linkers, the careful design of which can lead to novel materials with tunable properties. An approach to linker design is through its functionalization, namely the incorporation of functional groups on the backbone of the linker and the resulting MOF structure. Throughout this Thesis two approaches for the incorporation of functional groups on MOFs were explored in two different chapters: Pre-synthetic covalent functionalization of the organic linker (Chapter 2) and the incorporation of molecules with pre-registered functional groups on their molecular structures (Chapter 3). Our endeavors lead to novel materials, the characterization of which revealed intriguing properties such as stability over moisture and framework flexibility. Our results indeed highlight the importance of ligand functionalization not only with respect to the enhancement of properties such as adsorption but also for the discovery of novel structures.
Language English
Subject Flexibility
MOFs
Responsiveness
Αντίδραση σε εξωτερικά ερεθίσματα
Δομική ευκαμψία
Μεταλλο-Οργανικά Πλέγματα
Issue date 2023-07-27
Collection   School/Department--School of Sciences and Engineering--Department of Chemistry--Post-graduate theses
  Type of Work--Post-graduate theses
Permanent Link https://elocus.lib.uoc.gr//dlib/d/b/5/metadata-dlib-1689676891-906428-8418.tkl Bookmark and Share
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